Hyperfine Coupling in Colloidal n-Type ZnO Quantum Dots: Effects on Electron Spin Relaxation

Abstract
Colloidal semiconductor nanocrystals are excellent systems for exploring the fundamental properties of quantum-confined charge carriers. Tremendous progress has already been made in understanding the properties of electron-hole pairs (excitons) confined in colloidal quantum dots (QDs) using optical spectroscopic techniques.1-6 In contrast with charge carriers in QD electronic excited states, the properties of QDs containing excess carriers in their ground states have received substantially less attention.7-19 To date, the primary experimental probe of such charged QDs has been electronic absorption spectroscopy, in which low-energy intraband excitations can be used to define the carrier wave function.
Description
Keywords
Hyperfine Coupling, Colloidal n-Type ZnO Quantum Dots, Electron Spin Relaxation
Citation
Whitaker, K. M., Ochsenbein, S. T., Smith, A. L., Echodu, D. C., Robinson, B. H., & Gamelin, D. R. (2010). Hyperfine coupling in colloidal n-type ZnO quantum dots: effects on electron spin relaxation. The Journal of Physical Chemistry C, 114(34), 14467-14472. Doi: 10.1021/jp106356y